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Effective regeneration of thermally deactivated commercial V-W-Ti catalysts

Xuesong SHANG, Jianrong LI, Xiaowei YU, Jinsheng CHEN, Chi HE

Frontiers of Chemical Science and Engineering 2012, Volume 6, Issue 1, Pages 38-46 doi: 10.1007/s11705-011-1167-z

Abstract: Two types of regenerated solutions, namely NH Cl (1 mol/L) and dilute H SO (0.5 mol/L), were employedThe catalyst regenerated by aqueous NH Cl had a higher activity than that of the catalyst treated by dilute

Keywords： V2sub>O5sub>-WO3sub>/TiO2sub> catalysts thermal deactivation regeneration NH4sub>Cl dilute H2sub>SO4sub> solution

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Rh2sub>O3sub>/hexagonal CePO4sub> nanocatalysts for N2sub>O decomposition

Huan Liu, Zhen Ma

Frontiers of Chemical Science and Engineering 2017, Volume 11, Issue 4, Pages 586-593 doi: 10.1007/s11705-017-1659-6

Abstract: Hexagonal CePO nanorods were prepared by a precipitation method and hexagonal CePO nanowires were prepared by hydrothermal synthesis at 150 °C. Rh(NO ) was then used as a precursor for the impregnation of Rh O onto these CePO materials. The Rh O supported on the CePO nanowires was much more active for the catalytic decomposition of N O than the Rh O supported on CePO nanorods. The stability of both catalysts as a function of time on stream was studied and the influence of the co-feed (CO , O , H O or O /H O) on the N O decomposition was also investigated. The samples were characterized by N adsorption-desorption, inductively coupled plasma optical emission spectroscopy, X-ray diffraction, transmission electron microscopy, X-ray photoelectron microscopy, hydrogen temperature-programmed reduction, oxygen temperature-programmed desorption, and CO temperature-programmed desorption in order to correlate the physicochemical and catalytic properties.

Keywords： Rh2sub>O3sub> CePO4sub> N2sub>O decomposition

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ZnFe2sub>O4sub>/BiVO4sub> Z-scheme heterojunction for efficient visible-light photocatalytic

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 11, Pages 1728-1740 doi: 10.1007/s11705-023-2322-z

Abstract: A novel Z-scheme ZnFe2sub>O4sub>/BiVO4sub> heterojunction photocatalyst was successfullyCompared with the single-phase counterparts, ZnFe2sub>O4sub>/BiVO4sub> demonstratedConsequently, the 30% ZnFe2sub>O4sub>/BiVO4sub> catalyst afforded a degradation>4sub>-based catalysts.Moreover, the as-synthesized ZnFe2sub>O4sub>/BiVO4sub> heterojunctions were quite

Keywords： ZnFe2sub>O4sub>/BiVO4sub> Z-scheme heterojunction photocatalytic degradation

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ZnFe2sub>O4sub> deposited on BiOCl with exposed (001) and (010) facets for photocatalyticreduction of CO2sub> in cyclohexanol

Guixian Song, Xionggang Wu, Feng Xin, Xiaohong Yin

Frontiers of Chemical Science and Engineering 2017, Volume 11, Issue 2, Pages 197-204 doi: 10.1007/s11705-016-1606-y

Abstract: ZnFe O -BiOCl composites were prepared by both hydrothermal and direct precipitation processes and the structures and properties of the samples were characterized by various instrumental techniques. The samples were then used as catalysts for the photocatalytic reduction of CO in cyclohexanol under ultraviolet irradiation to give cyclohexanone (CH) and cyclohexyl formate (CF). The photocatalytic CO reduction activities over the hydrothermally prepared ZnFe O -BiOCl composites were higher than those over the directly-precipitated composites. This is because compared to the direct-precipitation sample, the ZnFe O nanoparticles in the hydrothermal sample were smaller and more uniformly distributed on the surface of BiOCl and so more heterojunctions were formed. Higher CF and CH yields were obtained for the pure BiOCl and BiOCl composite samples with more exposed (001) facets than for the samples with more exposed (010) facets. This is due to the higher density of oxygen atoms in the exposed (001) facets, which creates more oxygen vacancies, and thereby improves the separation efficiency of the electron-hole pairs. More importantly, irradiation of the (001) facets with ultraviolet light produces photo-generated electrons which is helpful for the reduction of CO to ·CO . The mechanism for the photocatalytic reduction of CO in cyclohexanol over ZnFe O -BiOCl composites with exposed (001) facets involves electron transfer and carbon radical formation.

Keywords： reduction of CO2sub> cyclohexanol ZnFe2sub>O4sub> deposited BiOCl facet composite

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Study on the performance of EDI device in dealing with Ni2 sub>solution with dilute departments

Niu Yubiao,Xu Xiaoqing,Zhao Haiyang,Zhou Zhijun

Strategic Study of CAE 2014, Volume 16, Issue 7, Pages 62-67

Abstract: filled with cation exchange resins and feed water was low concentration Ni2 sub>solution, forWith the feed solution whose Ni²⁺ sub> concentration was 50 mg·L^-1 and pH was 4.5, the results show that the out dilute Ni²⁺concentration was lower than 2mg·L^-1sub> and the Ni²⁺ concentration of out concentrate could higher;h^-1sub>.

Keywords： Electrodeionization (EDI) cation exchange resin heavy-metal Ni2 sub>

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VALORIZATION OF BIOGAS THROUGH SIMULTANEOUS CO AND HS REMOVAL BY RENEWABLE AQUEOUS AMMONIA SOLUTION IN

Frontiers of Agricultural Science and Engineering 2023, Volume 10, Issue 3, Pages 468-478 doi: 10.15302/J-FASE-2022473

Abstract:

● Simultaneous H2sub>S and CO2sub> removal from biogas

Keywords： biomethane biogas purification CO2sub> removal H2sub>S removal membrane absorption

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acid anions on highly efficient Ce-based catalysts for selective catalytic reduction of NO with NH3sub>

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 10, Pages 1399-1411 doi: 10.1007/s11705-023-2345-5

Abstract: Three kinds of Ce-based catalysts (CePO4sub>, CeVO4sub>, Ce2sub>(SO4sub>)The catalytic efficiencies of the three catalysts are as follow: CePO4sub> > CeVO4sub>> Ce2sub>(SO4sub>)3sub>, which is in agreement with their abilities of NH3sub>4sub>^3–, VO4sub>^3– and SO4sub>^2–2sub> for Ce2sub>(SO4sub>)3sub>.

Keywords： CePO4sub> CeVO4sub> Ce2sub>(SO4sub>)3sub> selective catalytic reduction

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Removal of P4sub>, PH3sub> and H2sub>S from Yellow Phosphoric Tail Gas by a Catalytic

Ning Ping,Hans-Jörg Bart,Wang Xueqian,Ma Liping,Chen Liang

Strategic Study of CAE 2005, Volume 7, Issue 6, Pages 27-35

Abstract: sulfide in yellow phosphorus tail gas was investigated with activated carbon and a home-made catalyst KU2.Both KU2 and activated carbon proved to be effective catalysts in the catalytic oxidation process (COP) for H2sub>S and PH3sub> removal.

Keywords： catalyst catalytic oxidation H2sub>S P4sub> PH3sub> fixed bed

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Frontier science and challenges on offshore carbon storage

Frontiers of Environmental Science & Engineering 2023, Volume 17, Issue 7, doi: 10.1007/s11783-023-1680-6

Abstract:

● The main direct seal up carbon options and challenges are reviewed.

Keywords： Offshore carbon storage Direct CO2sub> injection CO2sub>-CH4sub> replacement CO2sub>-EOR CCS hubs CO2sub> transport

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Removal of rhodamine B from aqueous solution by BiPO

Lei LI, Jian XU, Changsheng GUO, Yuan ZHANG

Frontiers of Environmental Science & Engineering 2013, Volume 7, Issue 3, Pages 382-387 doi: 10.1007/s11783-013-0504-5

Abstract: Hexahedron-like BiPO microcrystals were sucessfully synthesized via a template-free hydrothermal method. The resulting samples were characterized by X-ray diffraction (XRD), field-emission scanning electron microscopy (FESEM), transmission electron microscopy (TEM) and UV–vis spectroscopy. The BiPO samples were of pure monoclinic phase, and the initial amount of during synthesis did not show obvious effect on the phase properties of the materials. The hexahedron-like BiPO microcrystal had explicitly cut edges, and its thickness was about 1 μm. The photocatalytic performance of the BiPO catalysts was evaluated by photodegradation of RhB under UV light irradiation with commerial Degussa P25 TiO as reference. Compared with P25, the BiPO catalysts displayed higher photocatalytic activity, with 98.7% of RhB degraded during 60-min experiment. Cost evaluation analysis was adopted to describe the energy consumption of the degradation process, and the results suggested the potential application of this material in the field of dye-contaminated wastewater treatment or environmental matrices remediation.

Keywords： BiPO4sub> photocatalysis Rhodamine B cost evaluation

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CH4sub> and N2sub>O emissions from double-rice cropping system as affected by Chinese milk

Heshui XU,Dengyun LI,Bo ZHU,Kai ZHANG,Yadong YANG,Chen WANG,Ying JIANG,Zhaohai ZENG

Frontiers of Agricultural Science and Engineering 2017, Volume 4, Issue 1, Pages 59-68 doi: 10.15302/J-FASE-2017137

Abstract: Chinese milk vetch (CMV) and rice straw (RS) were incorporated into soil to substitute for synthetic N fertilizers and to maintain soil fertility. However, little is known about the integrated impacts of CMV and RS incorporation on CH and N O emissions in double-rice cropping systems in southern China. A field experiment was conducted to estimate the integrated impacts of CMV and RS incorporation in the early- and late-rice seasons on CH and N O emissions. All treatments received uniform N inputs, 6%–37% of which was replaced by CMV and RS crop residue. CMV and/or RS incorporation produced equivalent or slightly more grain yield, while reducing N O emissions by 3%–43%. However, both CMV and RS incorporation increased CH emissions. Annual CH emissions ranged from 321 to 614 kg·hm from CMV and RS amendment treatments, which were 1.5–2.9 times higher than that from synthetic N. Compared with single synthetic N fertilizer, incorporation of CMV and/or RS increased GWP and yield-scaled GWP by 45%–164% and 45%–153%, respectively. Our results demonstrate CMV and RS amendments replacing N fertilizer, maintained stable yield, mitigated N O emission, but enhanced CH emission. Further study is needed on crop residue management in double-cropping rice systems.

Keywords： Chinese milk vetch CH4sub> double-rice cropping system grain yield N2sub>O rice straw

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Complete oxidation of methane on CoO-SnO catalysts

Xingfu TANG , Jiming HAO , Junhua LI ,

Frontiers of Environmental Science & Engineering 2009, Volume 3, Issue 3, Pages 265-270 doi: 10.1007/s11783-009-0019-2

Abstract: CoO-SnO hybrid oxides were prepared by the coprecipitation method and were used to oxidate methane (CH) in presence of oxygen. The CoO-SnO with a molar ratio of Co/(Co+Sn) at 0.75 exhibited the highest catalytic activity among all the CoO-SnO hybrid oxides. Experimental results showed that the catalysts were considerably stable in the CH combustion reaction, and were verified by X-ray photoelectron spectra (XPS). It was found that CoO was the active species, and SnO acted as a support or a promoting component in the CoO-SnO hybrid oxides. The surface area was not a major factor that affected catalytic activity. The hydrogen temperature-programmed reduction (H-TPR) results demonstrated that the interaction between cobalt and tin oxides accelerated the mobility of oxygen species of CoO-SnO, leading to higher catalytic activity.

Keywords： Co3sub>O4sub>-SnO2sub> complete oxidation methane (CH4sub>)

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Ultrasound-assisted co-precipitation synthesis of mesoporous Co3O4–CeO2 composite oxides for highly selective

Frontiers of Chemical Science and Engineering 2022, Volume 16, Issue 8, Pages 1211-1223 doi: 10.1007/s11705-022-2145-3

Abstract: In this study, a Co3sub>O4sub>–CeO2sub> composite oxide catalyst was successfullyselectivity to KA-oil, which was benefited from the synergistic effects between Co³⁺/Co²⁺ and Ce⁴⁺/Ce³⁺ redox pairs, than bulk CeO2sub> and/or Co3sub>O4sub>.>3sub>O4sub>–CeO2sub>.

Keywords： Co3sub>O4sub>–CeO2sub> composite oxides cyclohexanone cyclohexanol ultrasonic-assisted

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Sulfur-deficient CoNi2sub>S4sub> nanoparticles-anchored porous carbon nanofibers as bifunctional

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 11, Pages 1707-1717 doi: 10.1007/s11705-023-2308-x

Abstract: >2sub>S4sub> nanoparticles are prepared as bifunctional electrocatalyst.>2sub>S4sub>.>2sub>S4sub> from 1.68 to 0.52 eV.Moreover, the uniform distribution of CoNi2sub>S4sub> nanoparticles on carbon nanofibersevolution reaction and 380 mV@100 mA·cm^–2 for hydrogen evolution reaction.

Keywords： nanoparticle sulfur vacancy porous carbon nanofiber transition metal sulfides electrolysis

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NiCo2O4@quinone-rich N–C core–shell nanowires as composite electrode for electric double layer capacitor

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 4, Pages 373-386 doi: 10.1007/s11705-022-2223-6

Abstract: >2sub>O4sub> nanowires were firstly grown on the substrate of active carbon cloth to provideThen, the quinone-rich nitrogen-doped carbon shell structure was formed around NiCo2sub>O4sub> nanowires, and the obtained composite was used as electrode for electric double layer capacitorresults showed that the composite electrode displayed an area-specific capacitance of 1794 mF∙cm^–2 at the current density of 1 mA∙cm^–2.

Keywords： carbon cloth NiCo2sub>O4sub> nanowires core−shell structure quinone-rich electric double

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Title Author Date Type Operation

Effective regeneration of thermally deactivated commercial V-W-Ti catalysts

Xuesong SHANG, Jianrong LI, Xiaowei YU, Jinsheng CHEN, Chi HE

Journal Article

Rh2sub>O3sub>/hexagonal CePO4sub> nanocatalysts for N2sub>O decomposition

Huan Liu, Zhen Ma

Journal Article

ZnFe2sub>O4sub>/BiVO4sub> Z-scheme heterojunction for efficient visible-light photocatalytic

Journal Article

ZnFe2sub>O4sub> deposited on BiOCl with exposed (001) and (010) facets for photocatalyticreduction of CO2sub> in cyclohexanol

Guixian Song, Xionggang Wu, Feng Xin, Xiaohong Yin

Journal Article

Study on the performance of EDI device in dealing with Ni2 sub>solution with dilute departments

Niu Yubiao,Xu Xiaoqing,Zhao Haiyang,Zhou Zhijun

Journal Article

VALORIZATION OF BIOGAS THROUGH SIMULTANEOUS CO AND HS REMOVAL BY RENEWABLE AQUEOUS AMMONIA SOLUTION IN

Journal Article

acid anions on highly efficient Ce-based catalysts for selective catalytic reduction of NO with NH3sub>

Journal Article

Removal of P4sub>, PH3sub> and H2sub>S from Yellow Phosphoric Tail Gas by a Catalytic

Ning Ping,Hans-Jörg Bart,Wang Xueqian,Ma Liping,Chen Liang

Journal Article

Frontier science and challenges on offshore carbon storage

Journal Article

Removal of rhodamine B from aqueous solution by BiPO

Lei LI, Jian XU, Changsheng GUO, Yuan ZHANG

Journal Article

CH4sub> and N2sub>O emissions from double-rice cropping system as affected by Chinese milk

Heshui XU,Dengyun LI,Bo ZHU,Kai ZHANG,Yadong YANG,Chen WANG,Ying JIANG,Zhaohai ZENG

Journal Article

Complete oxidation of methane on CoO-SnO catalysts

Xingfu TANG , Jiming HAO , Junhua LI ,

Journal Article

Ultrasound-assisted co-precipitation synthesis of mesoporous Co3O4–CeO2 composite oxides for highly selective

Journal Article

Sulfur-deficient CoNi2sub>S4sub> nanoparticles-anchored porous carbon nanofibers as bifunctional

Journal Article

NiCo2O4@quinone-rich N–C core–shell nanowires as composite electrode for electric double layer capacitor

Journal Article

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